Dongle Sonoff ZigBee 3.0 plus that I would like to use only as a router

+1

Upgrade coordinator firmware on ITead Sonoff ZigBee 3.0 Plus dongle on a seperate computer then migrate to it so it becomes the new Zigbee Coordinator before reflash your CC2531 with router firmware.

https://github.com/Koenkk/Z-Stack-firmwarehttps://github.com/Koenkk/Z-Stack-firmware/tree/master/router

Suggest that you also read/follow:

https://community.home-assistant.io/t/iteads-sonoff-zigbee-3-0-usb-dongle-plus-based-on-texas-instruments-cc2652p-20dbm-radio-mcu-now-sold-for-14-99/340705/